Please use this identifier to cite or link to this item: http://hdl.handle.net/20.500.11790/1519
Title: Multifunctional iron-carbon nanocomposites through an aerosol-based process for the in situ remediation of chlorinated hydrocarbons
Authors: Zhan, Jingjing 
Kolesnichenko, Igor 
Sunkara, Bhanukiran 
He, Jibao 
McPherson, Gary L. 
Piringer, Gerhard 
John, Vijay T. 
Issue Date: 2011
Publisher: American Chemical Society
Source: Environmental Science & Technology, 45(5), 1949-1954
Journal: Environmental Science & Technology 
Abstract: Spherical iron-carbon nanocomposites were developed through a facile aerosol-based process with sucrose and iron chloride as starting materials. These composites exhibit multiple functionalities relevant to the in situ remediation of chlorinated hydrocarbons such as trichloroethylene (TCE). The distribution and immobilization of iron nanoparticles on the surface of carbon spheres prevents zerovalent nanoiron aggregation with maintenance of reactivity. The aerosol-based carbon microspheres allow adsorption of TCE, thus removing dissolved TCE rapidly and facilitating reaction by increasing the local concentration of TCE in the vicinity of iron nanoparticles. The strongly adsorptive property of the composites may also prevent release of any toxic chlorinated intermediate products. The composite particles are in the optimal range for transport through groundwater saturated sediments. Furthermore, those iron-carbon composites can be designed at low cost, the process is amenable to scale-up for in situ application, and the materials are intrinsically benign to the environment.
URI: http://hdl.handle.net/20.500.11790/1519
ISSN: 0013-936X
DOI: 10.1021/es103493e
Rights: info:eu-repo/semantics/closedAccess
Appears in Collections:Energie-Umweltmanagement

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